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Sensitivity of coherent anti-Stokes Raman lineshape to time asymmetry of laser pulses

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Author

Summary, in English

We show that coherent anti-Stokes Raman lineshapes do not follow known spectral profiles if the time asymmetry of realistic laser pulses is taken into account. Examples are given for nanosecond and picosecond laser pulses commonly employed in frequency-resolved coherent anti-Stokes Raman scattering. More remarkably, the analysis suggests an effect of line narrowing in comparison to the customary approach, based primarily on the Voigt lineshape. (C) 2014 Optical Society of America

Department/s

Publishing year

2014

Language

English

Pages

5748-5751

Publication/Series

Optics Letters

Volume

39

Issue

19

Document type

Journal article

Publisher

Optical Society of America

Topic

  • Atom and Molecular Physics and Optics

Status

Published

ISBN/ISSN/Other

  • ISSN: 0146-9592